YIN Zhao-qin, LIN Jian-zhong, ZHOU Kun. Research on the Nucleation and Coagulation of Nanoparticles in the Parallel Twin Jets[J]. Applied Mathematics and Mechanics, 2008, 29(2): 140-148.
Citation: YIN Zhao-qin, LIN Jian-zhong, ZHOU Kun. Research on the Nucleation and Coagulation of Nanoparticles in the Parallel Twin Jets[J]. Applied Mathematics and Mechanics, 2008, 29(2): 140-148.

Research on the Nucleation and Coagulation of Nanoparticles in the Parallel Twin Jets

  • Received Date: 2006-05-16
  • Rev Recd Date: 2007-12-25
  • Publish Date: 2008-02-15
  • The large eddy simulation method has been used to simulate the diffusion of H2SO4 vapor in the parallel twin jets.The distributions of number concentration and size of nanoparticles produced by nucleation and coagulation in sulfuric acid/water system were given.The functions of the sulfur content,relative humidity and jet Reynolds number were evaluated according to the distributions of number concentration and size of nanoparticles.The results show that the nucleation in sulfuric acid/water system produces large number of nanoparticles,and ga-sto-nanoparticle conversion mostly takes place in the middle and interface of the twin jets.The coagulation process of particles reduces the number concentration but increases the mean particle size.For the case with higher sulfur content,more number and smaller size nanoparticles are produced by nucleation and coagulation.There is also a larger number of nanoparticles for the cases with higher relative humidity and jet Reynolds number.
  • loading
  • [1]
    Shi J P, Harrison R M. Investigation of ultrafine particle formation during diesel exhaust dilution[J].Environ Sci Technol,1999,33:3730-3736. doi: 10.1021/es981187l
    [2]
    于明州,林建忠,陈丽华.平面射流中纳米粒子积聚的矩方法[J].应用数学和力学,2007,28(11):1287-1295.
    [3]
    Kittelson D B. Engine and nanoparticles: a review[J].J Aerosol Sci,1998,29:575-588. doi: 10.1016/S0021-8502(97)10037-4
    [4]
    Yu M Z, Lin J Z,Chan T L.Numerical simulation of nanoparticle synthesis in diffusion flame reactor[J].Powder Technology,2007,180(1):9-20.
    [5]
    Friedlander S K, Wang C S.The self-preserving distribution for coagulation by Brownian motion[J].J Colloid Interface Sci,1966,22:126-132. doi: 10.1016/0021-9797(66)90073-7
    [6]
    Lai F S, Friedlander S K,Pich J,et al.The self-preserving particle size distribution for Brownian coagulation in the free-molecule regime[J].J Colloid Interface Sci,1972,39:395-405. doi: 10.1016/0021-9797(72)90034-3
    [7]
    Kulmala M, Laaksonen A,Pirjola L.Parameterizations for sulfuric acid/water nucleation rates[J].J Geophys,1998,103:8301-8309. doi: 10.1029/97JD03718
    [8]
    Vehkamaki H, Kulmala M,Lehtinen K E J,et al. Modelling binary homogeneous nucleation of water-sulfuric acid vapors: parameterisation for high temperature emissions[J].Environ Sci Technol,2003,37:3392-3398. doi: 10.1021/es0263442
    [9]
    Yin Z Q, Lin J Z, Zhou K,et al.Numerical simulation of the formation of pollutant nanoparticles in the exhaust twin-jet plume of a moving car[J].International Journal of Nonlinear Sciences and Numerical Simulation,2007,8(4):535-543.
    [10]
    Yin Z Q,Zhang H J, Lin J Z.Experimental study on the flow fleid characteristics in the mixing region of twin jets[J].Journal of Hydrodynamics, Ser B,2007,19(3):309-313. doi: 10.1016/S1001-6058(07)60063-8
    [11]
    Yu M Z, Lin J Z,Chen L H,et al.Large eddy simulation of a planar jet flow with nanoparticle coagulation[J].Acta Mechanica Sinica,2006,22(4):293-300. doi: 10.1007/s10409-006-0011-z
    [12]
    Smagorinsky J.General circulation experiments with the primitive equations[J].Mon Weather Rev,1963,91:91-164.
    [13]
    Deardorff J W.A numerical study of three-dimensional turbulent channel flow at large Reynolds numbers[J].J Fluid Mech,1970,41:453-480. doi: 10.1017/S0022112070000691
    [14]
    Lilly D K.A proposed modification of the germano subfrid-scale closure method[J].Phys Fluids,1993,4:633-635.
    [15]
    Friedlander S K.Smoke, Dust, and Haze, Fundamentals of Aerosol Dynamics[M].2nd Ed.New York:Oxford University Press,2000.
  • 加载中

Catalog

    通讯作者: 陈斌, bchen63@163.com
    • 1. 

      沈阳化工大学材料科学与工程学院 沈阳 110142

    1. 本站搜索
    2. 百度学术搜索
    3. 万方数据库搜索
    4. CNKI搜索

    Article Metrics

    Article views (2297) PDF downloads(491) Cited by()
    Proportional views
    Related

    /

    DownLoad:  Full-Size Img  PowerPoint
    Return
    Return